Kiss Kiss Bang Bang
Lost In Translation
In Bruges
Leon (The Professional)
Catch Me If You Can
The Shawshank Redemption is as good a movie as has ever been made.
It really is. It's one of the few movies that gets that kind of hype, and still exceeds expectations.
What about Bond films? I've only seen The World is Not Enough. The only reason I watched that one was because I lost my N64 cartridge and needed to know how it ended.
Connery: From Russia With Love, Goldfinger (You Only Live Twice isn't as good, but is still fun)
Lazenby: On Her Majesty's Secret Service
Dalton: The Living Daylights, License To Kill (TLD moreso, but LTK is really good too)
Brosnan: Goldeneye, Goldeneye, Goldeneye
Craig: Casino Royale (If you watch Quantum of Solace, try to watch it as soon as possible after CR. Your enjoyment of QoS will probably hinge heavily on that).
If I had to limit it to a top 5 (chronological ordder, not in order of quality);
From Russia With Love, OHMSS, The Living Daylights, Goldeneye, Casino Royale